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Havent read literally any of the other comments, since I didn't want to be biased.
Isaac can use items like The Mind and The Compass to find things that Voldemort has like horcruxes. Also, Blue Map would be able to find the room of requirement incase somehow voldemort stole an item or something, isaac could just get it back. I'll go through all the horcruxes.
1. The Diary. Isaac can use things like Scorpio, Serpents Kiss, or Common Cold to generate a poison to kill this one.
2. The Ring. Easy enough, just stab it with Sacrificial Dagger.
3. The Cup. Same thing again, use Dagger or Poison to destroy.
4. The Locket. Again, dagger or poison
5. The Diadem. Dagger or Poison...
6. The Harry. Isaac can kill Harry, easy.
7. The Snake. Sacrifical Dagger.
Theres also always Brimstone, Mom's Knife, Bombs, etc.
The killing part is easy too. He could deflect any projectiles with The Soul, and I think theres an item that makes him immune to lasers, which Avada Kedavra would count as. Even if not, with all those items, he gets something like 13 extra lives with a 50 percent chance of reviving anyway when out of extra lives. Also he has flight and stuff.