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Even though I don't believe the Time Gem would be relevant in this matchup due to AS's insane hax, I believe there's instances from the Marvel Comics where the IG was used against beings from other universes/dimensions invading the Marvel verse (Beyonders?) I haven't read those particular...
How strong is Tifa's BFR resistance? The Ruby Weapon can eject party members from battle with Whirlsand, which I don't recall any party member in VII having resistance to. If a mere sand tornado can BFR Tifa, then Marvel Comic Thanos's multiple ways of BFR (like opening a portal into space...
Even if Thanos isn't able to kill Chara for some reason, he can simply seal him like he did to the abstracts in Infinity Gauntlet.
Stomp in favor of Thanos
At both 2A, at a glance it looks like Nanashi would win due to superior hax. If they're both at their tier 1 forms (you did say at least 2A), Thanos just absorbs Nanashi.
Even base Thanos is quite powerful (4B), while Madara is 5B. Thanos stomps, especially with the wide array of technology he has at his disposal; he can simply send Madara into space with his portals, among other ways he can dispose of him.
Edit: Didn't notice it was MCU, I've only read the comics
I don't know why he even mentioned those characters, Thanos stomped on 10 tier 2C+ beings at once. Even someone with less experience with the gauntlet (his daughter Nebula) was able to do the same thing, and that time the beings had experience from fighting Thanos earlier so their strategy had...